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Pollution characteristics of particulate matters emitted from outdoor barbecue cooking in urban Jinan

Yifei Song, Lei Sun, Xinfeng Wang, Yating Zhang, Hui Wang, Rui Li, Likun Xue, Jianmin Chen, Wenxing Wang

《环境科学与工程前沿（英文）》 2018年 第12卷 第2期 doi: 10.1007/s11783-018-1024-0

摘要： To understand the pollution characteristics of particulate matter emitted from outdoor barbecue cooking in eastern China, measurements of the PM mass concentration, the number concentration of particles with a diameter of 0.01 to 1.0 m, and the particle size distribution from 0.3 to 25 m were carried out at seven barbecue restaurants in urban Jinan. The average PM mass concentration and sub-micron particle number concentrations at a distance of 1 m from the grills were 250 to 1083 g/m and 0.90 × 10 to 2.23 × 10 cm , respectively, which were much higher than those in the ambient air of the urban area. Compared to the ambient atmosphere, barbecue cooking emitted very high levels of particles with a larger increase in the concentrations of super-micron particles than that of sub-micron particles. The super-micron particle number concentrations at the barbecue restaurants were 10 to 100 times higher than those observed in the ambient urban atmosphere. The barbecue smoke had a significant effect on the particle concentrations in the surrounding region. Both mass and number concentrations of particles exhibited maximum values immediately near the barbecue grills and often reached a peak at a distance of 10 to 15 m. The removal efficiency of a range hood for the cooking particles was tested in an indoor kitchen. The range hood effectively cleaned the particulate matter pollution caused by cooking with a removal efficiency larger than 80%. Therefore, the use of a range hood is recommended for outdoor barbecue restaurants coupled with a smoke purifier to clean the emitted high concentrations of particles.To understand the pollution characteristics of particulate matter emitted from outdoor barbecue cooking in eastern China, measurements of the PM mass concentration, the number concentration of particles with a diameter of 0.01 to 1.0 m, and the particle size distribution from 0.3 to 25 m were carried out at seven barbecue restaurants in urban Jinan. The average PM mass concentration and sub-micron particle number concentrations at a distance of 1 m from the grills were 250 to 1083 g/m and 0.90 × 10 to 2.23 × 10 cm , respectively, which were much higher than those in the ambient air of the urban area. Compared to the ambient atmosphere, barbecue cooking emitted very high levels of particles with a larger increase in the concentrations of super-micron particles than that of sub-micron particles. The super-micron particle number concentrations at the barbecue restaurants were 10 to 100 times higher than those observed in the ambient urban atmosphere. The barbecue smoke had a significant effect on the particle concentrations in the surrounding region. Both mass and number concentrations of particles exhibited maximum values immediately near the barbecue grills and often reached a peak at a distance of 10 to 15 m. The removal efficiency of a range hood for the cooking particles was tested in an indoor kitchen. The range hood effectively cleaned the particulate matter pollution caused by cooking with a removal efficiency larger than 80%. Therefore, the use of a range hood is recommended for outdoor barbecue restaurants coupled with a smoke purifier to clean the emitted high concentrations of particles.

关键词： Barbecue smoke     Particulate matters     Pollution characteristics     Emissions     Removal    

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Effects of ambient temperature on regulated gaseous and particulate emissions from gasoline-, E10- and

Rencheng Zhu, Jingnan Hu, Liqiang He, Lei Zu, Xiaofeng Bao, Yitu Lai, Sheng Su

《环境科学与工程前沿（英文）》 2021年 第15卷 第1期 doi: 10.1007/s11783-020-1306-1

摘要： Abstract • Emissions from two sedans were tested with gasoline, E10 and M15 at 30°C and -7°C. • As the temperature decreased, the PM, PN and BC emissions increased with all fuels. • Particulate emissions with E10 and M15 were more sensitive to the temperature. • The PN and BC generated during cold start-up dominated those over the WLTC. Ambient temperature has substantial impacts on vehicle emissions, but the impacts may differ between traditional and alcohol gasolines. The objective of this study was to investigate the effects of temperature on gaseous and particulate emissions with both traditional and alcohol gasoline. Regulated gaseous, particle mass (PM), particle number (PN) and black carbon (BC) emissions from typical passenger vehicles were separately quantified with gasoline, E10 (10% ethanol and 90% gasoline by volume) and M15 (15% methanol and 85% gasoline by volume) at both 30°C and -7°C. The particulate emissions with all fuels increased significantly with decreased temperature. The PM emissions with E10 were only 48.0%–50.7% of those with gasoline at 30°C but increased to 59.2%-79.4% at -7°C. The PM emissions with M15 were comparable to those with gasoline at 30°C, but at -7°C, the average PM emissions were higher than those with gasoline. The variation trend of PN emissions was similar to that of PM emissions with changes in the fuel and temperature. At 30°C, the BC emissions were lower with E10 and M15 than with gasoline in most cases, but E10 and M15 might emit more BC than gasoline at -7°C, especially M15. The results of the transient PN and BC emission rates show that particulate emissions were dominated mainly by those emitted during the cold-start moment. Overall, the particulate emissions with E10 and M15 were more easily affected by ambient temperature, and the advantages of E10 and M15 in controlling particulate emissions declined as the ambient temperature decreased.

关键词： Particle mass     Particle number     Black carbon     Alcohol gasoline     Low temperature    

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PM10 emissions from industrial coal-fired chain-grate boilers

Xinghua Li, Junzan Han, Lei Duan

《环境科学与工程前沿（英文）》 2017年 第11卷 第6期 doi: 10.1007/s11783-017-0966-y

摘要： Industrial coal-fired boiler is an important air pollutant emission source in China. The chain-grate boiler is the most extensively used type of industrial coal-fired boiler. An electrical low-pressure impactor, and a Dekati Low Pressure Impactor were applied to determine mass and number size distributions of PM at the inlet and the outlet of the particulate emission control devices at six coal-fired chain-grate boilers. The mass size distribution of PM generated from coal-fired chain-grate boilers generally displays a bimodal distribution that contains a submicron mode and a coarse mode. The PM in the submicron mode for burning with raw coal contributes to 33%±10 % of PM emissions, much higher than those for pulverized boilers. And the PM in the submicron mode for burning with briquette contributes up to 86 % of PM emissions. Multiclones and scrubbers are not efficient for controlling PM emission. Their average collection efficiencies for sub-micron particle and super-micron particle are 34% and 78%, respectively. Operating conditions of industrial steam boilers have influence on PM generation. Peak of the submicron mode during normal operation period is larger than the start-up period.

关键词： coal-fired chain-grate boiler     PM10     size distribution     particulate emission control devices     size-dependent collection efficiency    

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Combustion and emission characteristics of a turbo-charged common rail diesel engine fuelled with diesel-biodiesel-DEE blends

Ni ZHANG, Zuohua HUANG, Xiangang WANG, Bin ZHENG

《能源前沿（英文）》 2011年 第5卷 第1期   页码 104-114 doi: 10.1007/s11708-011-0138-x

摘要： The combustion and emission characteristics of a turbo-charged, common rail diesel engine fuelled with diesel-biodiesel-DEE blends were investigated. The study reports that the brake-specific fuel consumption of diesel-biodiesel-DEE blends increases with increase of oxygenated fuel fractions in the blends. Brake thermal efficiency shows little variation when operating on different diesel-biodiesel-DEE blends. At a low load, the NO emission of the diesel-biodiesel-DEE blends exhibits little variation in comparison with the biodiesel fraction. The NO emission slightly increases with increase in the biodiesel fraction in diesel-biodiesel-DEE blends at medium load. However, the NO emission increases remarkably with increase of the biodiesel fraction at high load. Particle mass concentration decreases significantly with increase of the oxygenated-fuels fraction at all engine speeds and loads; particle number concentration decreases remarkably with increase of the oxygenated-fuels fraction. HC and CO emissions decrease with increasing oxygenated-fuels fraction in these blends.

关键词： Combustion     particulate emissions     diesel-biodiesel-DEE blend     diesel engine    

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Cylindrical particulate internal flows: A review

Lizhong HUANG, Xiang GAO, Jianzhong LIN

《机械工程前沿（英文）》 2012年 第7卷 第4期   页码 385-393 doi: 10.1007/s11465-012-0354-z

摘要：

The study of cylindrical particulate internal flows has wide industrial applicability hence received much attention. This article reviews the cylindrical particulate internal flows over the past twenty years. The research is related to the cylindrical particulate flows in the straight channel, curved channel and rotational channel. Finally, several open research issues have been identified.

关键词： cylindrical particulate flow     internal flow    

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A method for quantifying bias in modeled concentrations and source impacts for secondary particulate

Cesunica E. Ivey, Heather A. Holmes, Yongtao Hu, James A. Mulholland, Armistead G. Russell

《环境科学与工程前沿（英文）》 2016年 第10卷 第5期 doi: 10.1007/s11783-016-0866-6

摘要： A method for quantifying source impacts for secondary PM species is derived. The method provides estimates of bias in modeled concentrations. Adjusted concentrations match corresponding observations at monitored locations. Sources impacts on secondary species are estimated over the US for 20 sources. Community Multi-Scale Air Quality (CMAQ) estimates of sulfates, nitrates, ammonium, and organic carbon are highly influenced by uncertainties in modeled secondary formation processes, such as chemical mechanisms, volatilization, and condensation rates. These compounds constitute the majority of PM mass, and reducing bias in estimated concentrations has benefits for policy measures and epidemiological studies. In this work, a method for adjusting source impacts on secondary species is developed that provides estimates of source contributions and reduces bias in modeled concentrations compared to observations. The bias correction adjusts concentrations and source impacts based on the difference between modeled concentrations and observations while taking into account uncertainties at the location of interest; and it is applied both spatially and temporally. We apply the method over the US for 2006. The mean bias for initial CMAQ concentrations compared to observations is −0.28 (OC), 0.11 (NO ), 0.05 (NH ), and −0.08 (SO ). The normalized mean bias in modeled concentrations compared to observations was effectively zero for OC, NO , NH , and SO after applying the secondary bias correction. 10-fold cross-validation was conducted to determine the performance of the spatial application of the bias correction. Cross-validation performance was favorable; correlation coefficients were greater than 0.69 for all species when comparing observations and concentrations based on kriged correction factors. The methods presented here address model uncertainties by improving simulated concentrations and source impacts of secondary particulate matter through data assimilation. Secondary-adjusted concentrations and source impacts from 20 emissions sources are generated for 2006 over continental US.

关键词： Particulate matter     Source apportionment     Secondary particulate matter     Chemical transport modeling     Receptor modeling    

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Vanadium and molybdenum concentrations in particulate from Palermo (Italy): analytical methods using

Diana AMORELLO,Santino ORECCHIO

《环境科学与工程前沿（英文）》 2015年 第9卷 第4期   页码 605-614 doi: 10.1007/s11783-014-0703-8

摘要： The main purpose of this work was to develop a reliable method for the determination of vanadium (V) and molybdenum (Mo) in atmosphere particles or aerosols because they can not be readily measured using conventional techniques. For this research, 30 particulate samples were collected from five different stations located at Palermo, Italy. We used the catalytic adsorptive stripping voltammetry and differential pulsed voltammetry to measure V and Mo in atmospheric particulate, respectively. The represented method includes advantages of high sensitivity, high selectivity, simplicity, reproducibility, speed and low costs. The quantification limits for V and Mo are, respectively, 0.57 and 0.80 ng·m . The precision, expressed as relative standard deviation (RSD %), was about 2% for both metals. The mean recoveries of added V and Mo were about 99.5% and ranged from 97% to 101%. Vanadium concentrations in particulate samples collected in Palermo area ranged from 0.57 to 7.7 ng·m , while Mo concentrations were in the range 0.8–51 ng·m . In many cases the concentrations of two elements in the particulate samples fall below the detection limits. The mean concentrations for V and Mo in particulate samples, collected in Palermo area, were respectively 3.1 and 5.9 ng·m .

关键词： vanadium     molybdenum     particulate     voltammetry     Palermo    

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Recent advances of hydrogen production through particulate semiconductor photocatalytic overall water

《能源前沿（英文）》 2022年 第16卷 第1期   页码 49-63 doi: 10.1007/s11708-022-0817-9

摘要： Solar energy-driven photocatalytic water splitting has been investigated for decades to produce clean and renewable green hydrogen. In this paper, the cutting-edge research within the overall water splitting system is summarized from the one-step photocatalytic overall water splitting (POWS) system to the two-step system and the cocatalysts research in this field. In addition, the photocatalytic reaction engineering study is also reviewed which is crucial for future scale-up. This mini-review provides a picture of survey of recent progress of relevant overall water splitting system, with particular attention paid to material system and mechanistic breakthroughs, and highlights the challenge and opportunity of the current system.

关键词： photocatalysis     overall water splitting     hydrogen    

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Seasonal variations in leaf capturing of particulate matter, surface wettability and micromorphology

Huixia WANG, Hui SHI, Yangyang LI, Ya YU, Jun ZHANG

《环境科学与工程前沿（英文）》 2013年 第7卷 第4期   页码 579-588 doi: 10.1007/s11783-013-0524-1

摘要： The seasonal changes in leaf particulate matter (PM) accumulation, surface wettability and micromorphology in urban tree species, including ( . ), ( . ) and ( . ), were studied during a single growing season. The three species showed distinct seasonal trends in PM accumulation, increasing from spring to autumn (or winter) even during the rainy season, but at different rates. During the study, the leaf PM retention amount of , a species with ridged leaf surfaces, was significantly higher than that of and , species with waxy leaf surfaces. The contact angles of water droplets on leaves decreased with leaf age except on the abaxial surface of , which remained non-wettable or highly non-wettable throughout the growing season; the decrease in the contact angle on adaxial surface of was greater when compared with and . A significant and negative relationship existed between leaf PM retention amounts and contact angles on adaxial surface of leaves of all three species. The increase in wettability, probably caused when epicuticular wax was destroyed by mechanical and chemical abrasion, seemed to be the main factor leading to seasonal variations in leaf PM accumulation.

关键词： contact angle     particulate matter     retention amount    

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Correlation between carbon emissions and energy structure –Reliability analysis of low carbon target

Ben HUA

《能源前沿（英文）》 2011年 第5卷 第2期   页码 214-220 doi: 10.1007/s11708-010-0133-7

摘要： The influence of energy intensity on carbon intensity depends upon the fraction of energy mixes with high carbon emissions in the total energy mixes . The correlation of with a variety of primary energy mix fractions and technology advances such as CCS and CCHP is analyzed and deduced. Taking the long-term carbon reduction target in 2050 settled upon by the Copenhagen Agreement and the mid-term target suggested by the “450 Scenes Program” of the International Energy Agency (IEA) as constraints, the new pattern of the energy transition of the world in 2020, 2030, and 2050 are estimated and figured out. The peak value of energy consumption will lag behind the peak value of carbon emissions; the world energy structure shifting point will be in 2020–2025. Estimates show that China’s mid-2020 and long-term targets of energy-saving and emission reduction announced by the Chinese government might be achieved.

关键词： correlation     carbon emissions     energy consumption     high carbon emissions energy mix     target of emission reduction     reliability    

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Determination of polyfluoroalkyl compounds in water and suspended particulate matter in the river Elbe

Lutz AHRENS, Merle PLASSMANN, Zhiyong XIE, Ralf EBINGHAUS

《环境科学与工程前沿（英文）》 2009年 第3卷 第2期   页码 152-170 doi: 10.1007/s11783-009-0021-8

摘要： The distribution of polyfluoroalkyl compounds (PFCs) in the dissolved and particulate phase and their discharge from the river Elbe into the North Sea were studied. The PFCs quantified included C -C perfluorinated sulfonates (PFSAs), 6∶2 fluorotelomer sulfonate (6∶2 FTS), C and C perfluorinated sulfinates (PFSiAs), C -C perfluorinated carboxylic acids (PFCAs), perfluoro-3,7-dimethyl-octanoic acid (3,7m -PFOA), perfluorooctane sulfonamide (FOSA), and n-ethyl perfluroctane sulfonamidoethanol (EtFOSE). PFCs were mostly distributed in the dissolved phase, where perfluorooctanoic acid (PFOA) dominated with 2.9-12.5 ng/L. In the suspended particulate matter FOSA and perfluorooctane sulfonate (PFOS) showed the highest concentrations (4.0 ng/L and 2.3 ng/L, respectively). The total flux of ∑PFCs from the river Elbe was estimated to be 802 kg/year for the dissolved phase and 152 kg/year for the particulate phase. This indicates that the river Elbe acts as a source of PFCs into the North Sea. However, the concentrations of perfluorobutane sulfonate (PFBS) and perfluorobutanoic acid (PFBA) in the North Sea were higher than that in the river Elbe, thus an alternative source must exist for these compounds.

关键词： polyfluoroalkyl compounds (PFCs)     perfluorooctane sulfonate (PFOS)     perfluorooctanoic acid (PFOA)     surface water     water-particulate partitioning    

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Concentrations of toxic heavy metals in ambient particulate matter in an industrial area of northeastern

PIAO Fengyuan, SUN Xiance, LIU Shuang, YAMAUCHI Toru

《医学前沿（英文）》 2008年 第2卷 第2期   页码 207-210 doi: 10.1007/s11684-008-0040-z

摘要： This paper investigates concentrations of various heavy metals in ambient particulate matter (PM) and provide evidence for prevention from air pollution. The concentrations of heavy metal components in the PM were determined by inductively coupled plasma/Mass spectrometry (ICP/MS) from September 2000 to August 2002 in a northeast industrial city in China. Concentrations of Cd, Mn, Pb, Ni, Cr and As in the PM were 9.3, 461.9, 588.7, 69.5, 205.7 and 57.4 ng/m in the industrial area, and 5.7, 245.5, 305.0, 31.4, 58.8 and 32.5 ng/m in the main road, respectively. Concentrations of these heavy metals except Cd were significantly higher in the industrial area and main road than those in the suburban area ( < 0.05 or < 0.01). The change curves of the six heavy metal concentrations show their concentrations increased in the winter and spring, but decreased in the summer and autumn. The results indicate that concentrations of the metals in the PM are relatively high in the industrial area and main road.

关键词： summer     August     northeast industrial     September     spring    

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On the applicability of different adhesion models in adhesive particulate flows

Guanqing LIU, Shuiqing LI, Qiang YAO,

《能源前沿（英文）》 2010年 第4卷 第2期   页码 280-286 doi: 10.1007/s11708-009-0062-5

摘要： An adhesion map provides quantitative criteria for the appropriate selection of adhesion models applicable to a specific adhesive contact problem of fine particles in complex particulate flows. In this paper, three different general adhesion models are used to construct adhesion maps. The applicable regimes on the adhesion map for different approximate adhesion models are determined according to their underlying limitations. It is found that the choice of general model has limited influence on the structure of a constructed adhesion map. On the contrary, the regime of application for each approximate model is sensitive to the approximation level. A three-dimensional, more intuitive adhesion map based on physical parameters of particles is also built. Finally, recent applications of adhesion models in discrete element method (DEM) investigations of fine-particle flow dynamics are briefly discussed.

关键词： adhesive contact     van der Waals force     adhesion model     adhesion map     DEM    

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Particulate matter and metals partitioning in highway rainfall-runoff

Gaoxiang YING, John J. SANSALONE,

《环境科学与工程前沿（英文）》 2010年 第4卷 第1期   页码 35-46 doi: 10.1007/s11783-010-0009-4

摘要： This study investigated the particulate matter (PM) and metals in highway dry deposition and rainfall-runoff as a function of hydrologic transport and settling on an event basis. Events were differentiated as mass-limited (ML) and flow-limited (FL). Results indicate that unique and separate suspended sediment concentration (SSC) relationships with turbidity occurred for ML and FL events. Sixty minutes of quiescent settling produced a single SSC-turbidity relationship for all events. ML events transport higher proportions of settleable and sediment PM while FL events transported relatively higher suspended PM. For batch clarification with one hour of settling, ML events had generally higher treatment efficiencies compared to FL events for the same settling conditions. Highway dry deposition PM was hetero-disperse and coarse ( = 304 µm). Results indicate that the acidic rainfall is not a significant contributor to metals in runoff but is capable of leaching metals from dry deposition PM into runoff. Partitioning in retained runoff resulted in a particulate-bound €predominance €for €most €metals €except Ca and Mg. While the finer fraction of dry deposition PM (<75µm) generates the highest metal concentrations, the highest metal mass is associated with the coarser fraction (>75µm).

关键词： stormwater     particulate matter (PM)     turbidity     suspended sediment concentration (SSC)     unit operations     metals     dry deposition     acid rain    

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Reducing CO emissions from the rebalancing operation of the bike-sharing system in Beijing

《工程管理前沿（英文）》 2023年 第10卷 第2期   页码 262-284 doi: 10.1007/s42524-021-0168-y

摘要： With the development of the bike-sharing system (BSS) and the introduction of green and low carbon development, the environmental impacts of BSS had received increasing attention in recent years. However, the emissions from the rebalancing of BSS, where fossil-fueled vehicles are commonly used, are usually neglected, which goes against the idea of green travel in a sharing economy. Previous studies on the bike-sharing rebalancing problem (BRP), which is considered NP-hard, have mainly focused on algorithm innovation instead of improving the solution model, thereby hindering the application of many existing models in large-scale BRP. This study then proposes a method for optimizing the CO2 emissions from BRP and takes the BSS of Beijing as a demonstration. We initially analyze the spatial and temporal characteristics of BSS, especially the flow between districts, and find that each district can be independently rebalanced. Afterward, we develop a rebalancing optimization model based on a partitioning strategy to avoid deciding the number of bikes being loaded or unloaded at each parking node. We then employ the tabu search algorithm to solve the model. Results show that (i) due to over launch and lack of planning in rebalancing, the BSS in Beijing shows great potential for optimization, such as by reducing the number of vehicle routes, CO2 emissions, and unmet demands; (ii) the CO2 emissions of BSS in Beijing can be reduced by 57.5% by forming balanced parking nodes at the end of the day and decreasing the repetition of vehicle routes and the loads of vehicles; and (iii) the launch amounts of bikes in specific districts, such as Shijingshan and Mentougou, should be increased.

关键词： bike-sharing     CO2 emissions     environmental benefit     partitioning strategy     rebalancing problem    

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标题 作者 时间 类型 操作

Pollution characteristics of particulate matters emitted from outdoor barbecue cooking in urban Jinan

Yifei Song, Lei Sun, Xinfeng Wang, Yating Zhang, Hui Wang, Rui Li, Likun Xue, Jianmin Chen, Wenxing Wang

期刊论文

Effects of ambient temperature on regulated gaseous and particulate emissions from gasoline-, E10- and

Rencheng Zhu, Jingnan Hu, Liqiang He, Lei Zu, Xiaofeng Bao, Yitu Lai, Sheng Su

期刊论文

PM10 emissions from industrial coal-fired chain-grate boilers

Xinghua Li, Junzan Han, Lei Duan

期刊论文

Combustion and emission characteristics of a turbo-charged common rail diesel engine fuelled with diesel-biodiesel-DEE blends

Ni ZHANG, Zuohua HUANG, Xiangang WANG, Bin ZHENG

期刊论文

Cylindrical particulate internal flows: A review

Lizhong HUANG, Xiang GAO, Jianzhong LIN

期刊论文

A method for quantifying bias in modeled concentrations and source impacts for secondary particulate

Cesunica E. Ivey, Heather A. Holmes, Yongtao Hu, James A. Mulholland, Armistead G. Russell

期刊论文

Vanadium and molybdenum concentrations in particulate from Palermo (Italy): analytical methods using

Diana AMORELLO,Santino ORECCHIO

期刊论文

Recent advances of hydrogen production through particulate semiconductor photocatalytic overall water

期刊论文

Seasonal variations in leaf capturing of particulate matter, surface wettability and micromorphology

Huixia WANG, Hui SHI, Yangyang LI, Ya YU, Jun ZHANG

期刊论文

Correlation between carbon emissions and energy structure –Reliability analysis of low carbon target

Ben HUA

期刊论文

Determination of polyfluoroalkyl compounds in water and suspended particulate matter in the river Elbe

Lutz AHRENS, Merle PLASSMANN, Zhiyong XIE, Ralf EBINGHAUS

期刊论文

Concentrations of toxic heavy metals in ambient particulate matter in an industrial area of northeastern

PIAO Fengyuan, SUN Xiance, LIU Shuang, YAMAUCHI Toru

期刊论文

On the applicability of different adhesion models in adhesive particulate flows

Guanqing LIU, Shuiqing LI, Qiang YAO,

期刊论文

Particulate matter and metals partitioning in highway rainfall-runoff

Gaoxiang YING, John J. SANSALONE,

期刊论文

Reducing CO emissions from the rebalancing operation of the bike-sharing system in Beijing

期刊论文